The decay law for radioactive decay is given by the equation:
\[
N = N_0 e^{-\lambda t},
\]
where \( N \) is the number of nuclei at time \( t \), \( N_0 \) is the initial number of nuclei, and \( \lambda \) is the decay constant.
For nucleus \( n_2 \), the decay constant is 3 times that of \( n_1 \). So, the decay constants are:
\[
\lambda_2 = 3 \lambda_1.
\]
The number of nuclei after time \( t \) for both nuclei will be:
\[
N_2 = N_0 e^{-\lambda_2 t} = N_0 e^{-3\lambda_1 t},
\]
\[
N_1 = N_0 e^{-\lambda_1 t}.
\]
Now, after one half-life of \( n_1 \), the value of \( t = t_{\text{half}} \) is:
\[
t_{\text{half}} = \frac{\ln 2}{\lambda_1}.
\]
At this time, the number of nuclei for \( n_1 \) is:
\[
N_1 = N_0 e^{-\lambda_1 t_{\text{half}}} = \frac{N_0}{2}.
\]
For \( n_2 \), the number of nuclei after one half-life of \( n_1 \) is:
\[
N_2 = N_0 e^{-3\lambda_1 t_{\text{half}}} = N_0 e^{-\frac{3\ln 2}{\lambda_1}} = \frac{N_0}{2^3} = \frac{N_0}{8}.
\]
Thus, the ratio of the number of nuclei of \( n_2 \) to the number of nuclei of \( n_1 \) is:
\[
\frac{N_2}{N_1} = \frac{\frac{N_0}{8}}{\frac{N_0}{2}} = \frac{1}{4}.
\]
Thus, the correct answer is:
\[
\boxed{\frac{1}{4}}.
\]