To calculate the gain percentage:
1. Let the cost price of 100 pencils be $100x$.
2. The selling price of 60 pencils is also $100x$.
3. Therefore, the selling price of 100 pencils is $_frac{100x}{60} _times 100 = _frac{500x}{3}$.
The gain is calculated as:
_[
_text{Gain} = _frac{_text{Selling Price} - _text{Cost Price}}{_text{Cost Price}} _times 100_%
_]
_[
_text{Gain} = _frac{_frac{500x}{3} - 100x}{100x} _times 100_% = _frac{200x}{3x} _times 100_% = 66 _frac{2}{3} _%
_]
Therefore, the correct answer is (2) $66 _frac{2{3} _%$}.